Authors

  • J. Mirsultonov
    Pharmaceutical Education and Research Institute
  • S. Saidov
    Pharmaceutical Education and Research Institute,
  • Sh. Xolliyeva
    Pharmaceutical Education and Research Institute

DOI:

https://doi.org/10.71337/inlibrary.uz.jmsi.111685

Abstract

This article presents the results of laboratory testing of the antidote properties of the supramolecular compound methylene blue and hydroxypropyl beta-cyclodextrin for carbon monoxide poisoning.


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EXPERIMENTAL STUDY OF THE EFFECTIVENESS OF THE SUPRAMOLECULAR

COMPOUND OF METHYLENE BLUE AND HYDROXYPROPYL BETA-

CYCLODEXTRIN IN CARBON MONOXIDE POISONING

Sh.O.Xolliyeva, S.A.Saidov, J.A.Mirsultonov

Pharmaceutical Education and Research

Institute, Tashkent, Republic of Uzbekistan

Annotation:

This article presents the results of laboratory testing of the antidote properties of the

supramolecular compound methylene blue and hydroxypropyl beta-cyclodextrin for carbon

monoxide poisoning.

Keywords:

Methylene blue (MB), carbon monoxide (CO), cyanide and nitrate poisoning,

laboratory rat, hemoglobin, carboxyhemoglobin, effective antidote.

Introduction.

According to statistics, carbon monoxide poisoning is the second leading cause of death in the

world after alcohol poisoning. According to the Ministry of Emergency Situations, in Uzbekistan

in 2021, 125 people died from carbon monoxide poisoning, 115 were injured, and in 2022 this

figure reached 146 deaths and more than 50 injuries. Since the beginning of 2024, a total of 74

gas-related incidents have occurred in Uzbekistan (86 in 2023), resulting in 82 deaths and 80

injuries of varying degrees. In some cases, entire family members have died from carbon

monoxide poisoning due to a faulty chimney. As can be seen from the above, carbon monoxide

poisoning is common among the population, but unfortunately, these cases often end tragically.

Main part

Let's briefly talk about what carbon monoxide poisoning is and how the gas is formed. Carbon

monoxide is a strong poison, because it forms strong complexes with biologically active

molecules containing metal atoms (blood proteins, hemoglobin), which disrupts the oxygen

supply of tissues. It especially affects the cells of the central nervous system. The binding of

carbon monoxide to the Fe atoms in the hemoglobin protein disrupts the formation of

oxyhemoglobin, which carries oxygen from the lungs to the tissues. Even if there is 0.1% CO gas

in the air, this gas displaces half of the oxygen from oxyhemoglobin. In such cases, even the

presence of a large amount of pure oxygen in the air cannot prevent death from asphyxiation.

The daily permissible dose of carbon monoxide in atmospheric air is set at 3 mg / m³. In many

places in the workplace and public transport, it is 20 mg / m³. This gas is released into the air as

part of volcanic and swamp gases, and by the secretions of plankton and other microorganisms.

Thus, 220 million tons of CO are released into the atmosphere from the surface layers of the

ocean every year. In addition, large amounts of carbon monoxide are released into the air from

coal mines and forest fires. 300.4 thousand tons of CO are also released during the smelting of

every million tons of steel. In total, the annual release of man-made CO into the air is 600

million tons.

Based on the above, it is very important to develop alternative medical treatments for patients

with carbon monoxide poisoning. Traditional treatment methods (hyperbaric oxygen therapy) are

expensive and have limitations in providing rapid relief. Methylene blue (MK) converts COHb to

normal Hb, but its toxicity and low solubility limit its clinical application. In this study, the

antidote properties of the supramolecular compound MK+HP-β-CD were experimentally

investigated.

Research methods used based on the comments.


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Experimental group:

12 healthy male rats (Sprague-Dawley yoki Wistar)

Experimental group (n=6):

Lung saturation was measured and recorded using a specialized

veterinary Berry AM6200 Capnograph pulse oximeter for animals administered CO poisoning +

MB+HP-β-CD solution.

Control group (n=6):

Animals exposed to CO poisoning + saline were monitored for pulmonary

saturation using a Berry AM6200 Capnograph pulse oximeter. The duration of the experiment

was 1 day. Before the start of the experiment, the laboratory rats were named and their weight

was measured and recorded using an analytical scale. A special animal-safe alcohol-based

yellow dye was used to clearly distinguish the laboratory rats. The dye was used to label the rats'

tail, head, spine, left leg, left arm, right leg, right arm, left and right flanks, and neck. The Berry

AM6200 Capnograph was used and saturation and pulse were determined for 5 minutes, 1, 3, 6,

12, and 24 hours. 5 minutes after the animals were exposed to carbon monoxide, the pulse and

saturation of the animals in the control group did not differ from the experimental group. One

hour after poisoning the animals with carbon monoxide, the saturation in the experimental

animals was 10% higher and the pulse rate was 8% higher than in the control group. After 3

hours, the saturation was 20% higher and the pulse rate was 12%. 24 hours after poisoning the

animals and the introduction of 0.5% methylene blue, the saturation was on average 90%, the

pulse rate was 100 beats per minute. Compared with the results of the animals in the control

group, the saturation in the experimental group was restored faster, the pulse rate was within

normal limits. The result shows that the injection of 0.5% methylene blue saturates the blood

with oxygen and relieves the div from carbon monoxide poisoning.

Lung saturation and pulse in animals that received the poisoned injection and those that

did not.

Time after poisoning.

5 min

1 hour

3 hour

24 hour

№ Name

weight SpO2 % /

PR/bPm

SpO2 % /

PR/bPm

SpO2 % /

PR/bPm

SpO2 % /

PR/bPm

Ex

pe

rim

en

ta

lg

ro

up

(in

je

ct

ed

)

1

Head

215

40/40

48/127

69/110

93/127

2

Neck

225

39/25

51/89

67/98

89/143

3

spine

200

35/64

61/134

73/107

96/138

4

waist

220

36/56

57/118

76/113

87/146

5

Left hand

195

35/48

54/113

64/107

90/131

6

Right hand 225

38/58

59/121

79/126

91/118

Co

nt

ro

l

gr

ou

p

(n

o

in

je

ct

io

n)

7

Left hand

210

36/46

41/146

57/158

Death

recorded

8

Right foot 185

35/50

Death

recorded

-

-

9

Left

215

39/58

43/134

55/146

67/114


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Conclusions and results.

The supramolecular compound MK+HP-β-CD is an effective antidote

for CO poisoning, restoring SpO₂ to 90% within 24 hours.

HP-β-CD increases the solubility of MK and reduces its toxicity. The results can serve as a basis

for clinical trials. By studying the changes occurring in the div and analyzing them in depth, it

will be possible to develop alternative treatment methods for carbon monoxide poisoning.

References

.

1.

WHO. (2021). Carbon Monoxide Poisoning: Clinical

Management.

2.

Thom, S.R. (2011). Am J Physiol, 301(6), H1784-H1792.

3.

OʻzR Sogʻliqni Saqlash Vazirligi. (2024). Zaharlanish

Holatlari Hisoboti.

4.

Yangi

farmakologik

moddalarni

eksperimental

(klinikgacha) o'rganish bo'yicha uslubiy ko'rsatmalar. Rossiya Tibbiyot fanlari akademiyasining

muxbir aʼzosi, professor R. U. XABRIEVning umumiy tahriri ostida. Ikkinchi nashr, qayta ko'rib

chiqilgan va kengaytirilgan. M.: - 2005. - M.: "Nashriyot" OAJ "Tibbiyot", 2005. - 830 b.

5.

Belenkiy M.L. Farmakologik ta'sirni miqdoriy baholash

elementlari. L Medgiz 1963, -152 b.

6.

Ryaxovskiy

Andrey

Evgenievich

’’Alkogollik

intoksikasiyasi fonida kalamushlarni is gazi bilan zaharlanishni organizmda morfofunksional

o’zgarishi’’ Rossiya Federatsiyasi Sog'liqni saqlash vazirligining "Bashkir davlat tibbiyot

universiteti

7.

Novelli, P. C. (1999). CO in the atmosphere: measurement

techniques and related issues. Chemosphere — Global Change Science, 1(1-3), 115—126,

https://doi.org/10.1016/S1465-9972(99)00013-6

8.

Changes of Nuclear Factor Kappa-B Pathway Activity in

Hippocampus After Acute Carbon Monoxide Poisoning and Its Role in Nerve Cell Injury.

9.

Changes of Nuclear Factor Kappa-B Pathway Activity in

Hippocampus After Acute Carbon Monoxide Poisoning and Its Role in Nerve Cell Injury.

buttock

10 Right

buttock

195

42/68

47/145

58/183

69/135

11 Head/back 230

35/54

39/137

Death

recorded

-

12 Head/spine 210

39/56

45/87

61/114

73/156

References

WHO. (2021). Carbon Monoxide Poisoning: Clinical Management.

Thom, S.R. (2011). Am J Physiol, 301(6), H1784-H1792.

OʻzR Sogʻliqni Saqlash Vazirligi. (2024). Zaharlanish Holatlari Hisoboti.

Yangi farmakologik moddalarni eksperimental (klinikgacha) o'rganish bo'yicha uslubiy ko'rsatmalar. Rossiya Tibbiyot fanlari akademiyasining muxbir aʼzosi, professor R. U. XABRIEVning umumiy tahriri ostida. Ikkinchi nashr, qayta ko'rib chiqilgan va kengaytirilgan. M.: - 2005. - M.: "Nashriyot" OAJ "Tibbiyot", 2005. - 830 b.

Belenkiy M.L. Farmakologik ta'sirni miqdoriy baholash elementlari. L Medgiz 1963, -152 b.

Ryaxovskiy Andrey Evgenievich ’’Alkogollik intoksikasiyasi fonida kalamushlarni is gazi bilan zaharlanishni organizmda morfofunksional o’zgarishi’’ Rossiya Federatsiyasi Sog'liqni saqlash vazirligining "Bashkir davlat tibbiyot universiteti

Novelli, P. C. (1999). CO in the atmosphere: measurement techniques and related issues. Chemosphere — Global Change Science, 1(1-3), 115—126, https://doi.org/10.1016/S1465-9972(99)00013-6

Changes of Nuclear Factor Kappa-B Pathway Activity in Hippocampus After Acute Carbon Monoxide Poisoning and Its Role in Nerve Cell Injury.

Changes of Nuclear Factor Kappa-B Pathway Activity in Hippocampus After Acute Carbon Monoxide Poisoning and Its Role in Nerve Cell Injury.