Authors

  • Dilyora Sherbutayeva
    Almalyk branch of Tashkent State Technical University named after Islam Karimov
  • Kholida Azizova
    Almalyk branch of Tashkent State Technical University named after Islam Karimov

DOI:

https://doi.org/10.71337/inlibrary.uz.jmsi.123993

Abstract

This article examines the sorption process of rhenium (Re) and its effective methods. Due to the presence of perrhenate ions (ReO₄⁻) in industrial waste and the environment, which pose ecological risks, their efficient removal is one of the key challenges. Various types of sorbents, including activated carbon, ion-exchange sorbents, zeolites, and biomass-based materials, are analyzed. The main mechanisms of the sorption process, such as electrostatic forces, ion exchange, and Van der Waals interactions, are discussed. Furthermore, technologies for rhenium recovery using modern nanomaterials and modified polymers are explored. This review serves as a valuable source of information for research aimed at reducing rhenium's environmental hazards and developing effective purification methods.


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SORPTION OF RHENIUM: RESEARCH, METHODS, AND SCIENTIFIC

APPROACHES

Dilyora Dilshod kizi Sherbutayeva,

Kholida Mumin kizi Azizova

student, associate Professor, PhD in Chemical Sciences

Almalyk branch of Tashkent State Technical University named after Islam Karimov

dilyorasherbutayeva@gmail.com

Abstract:

This article examines the sorption process of rhenium (Re) and its effective methods.

Due to the presence of perrhenate ions (ReO₄⁻) in industrial waste and the environment, which

pose ecological risks, their efficient removal is one of the key challenges. Various types of

sorbents, including activated carbon, ion-exchange sorbents, zeolites, and biomass-based

materials, are analyzed. The main mechanisms of the sorption process, such as electrostatic

forces, ion exchange, and Van der Waals interactions, are discussed. Furthermore, technologies

for rhenium recovery using modern nanomaterials and modified polymers are explored. This

review serves as a valuable source of information for research aimed at reducing rhenium's

environmental hazards and developing effective purification methods.

Keywords

: rhenium sorption, perrhenate ions, sorption methods, activated carbon, ion-exchange

sorbents, zeolites, biomass, environmental purification, bioaccumulation, nanomaterials.

Introduction

The effective removal of rhenium (ReO₄⁻) from the environment and industrial waste is an

essential aspect of ecological purification. Due to rhenium’s high toxicity and radioactive

properties, its presence in water and soil may pose serious threats to the environment and human

health. Several methods are available for removing rhenium; however, sorption—i.e., adsorption

of rhenium onto a solid phase—is considered one of the most effective and economically viable

technologies. This article reviews scientific research and principal approaches related to rhenium

sorption.

Environmental Impact and Sources of Rhenium

Rhenium is primarily known as a decay product of ruthenium (Ru) isotopes found in radioactive

materials or resulting from industrial processes. Its high toxicity and long environmental

persistence increase its ecological risk. Accumulation of rhenium in water or soil may lead to

uptake by plants, subsequent transfer to animals, and entry into the human food chain, thus

posing health risks. Therefore, effective removal of rhenium and its separation from the

environment is crucial.

Methods of Rhenium Removal

Several methods are used for the removal of rhenium, including:


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Chemical Reduction

: Rhenium can be removed by changing its oxidation state, e.g.,

reducing Re(VII) to Re(IV). This process helps convert rhenium to other chemical forms, though

its effectiveness can sometimes be limited.

Filtration and Distillation

: These techniques are employed to remove rhenium from

liquids but often involve high energy consumption and time.

Sorption

: The sorption method, in which rhenium is adsorbed onto a solid phase, is

widely used and considered the most promising approach for removing rhenium from water and

other solutions.

Sorbents and Their Properties

Various materials are used as sorbents for removing rhenium. Effective sorbents typically have

high surface areas and chemical structures that allow for efficient rhenium adsorption. The most

commonly used sorbents include:

Activated Carbon

: This material has excellent adsorption properties and is effective in

perrhenate (ReO₄⁻) sorption. Its high surface area and porous structure enhance its sorption

efficiency [1].

Zeolites

: Natural minerals with microstructures and high surface areas that allow for

effective rhenium adsorption. They are chemically stable and environmentally friendly materials

[2].

Ion-Exchange Sorbents

: Polymer-based sorbents, especially sulfonated polymers,

operate via ion exchange. These resins are effective in rhenium sorption as they serve as electron

donors and accommodate large ions [3].

Modified Biomass

: Biomass materials derived from soil or plants can be chemically

modified to efficiently adsorb rhenium. These materials are environmentally benign and cost-

effective [4].

Sorption Processes and Mechanisms

The sorption of rhenium is based on several physicochemical mechanisms, including:

Electrostatic Forces

: Ionic properties of the sorbent surface facilitate adsorption of

rhenium as an anion. Electrostatic attraction helps bind rhenium to the solid phase [5].

Ion Exchange

: In ion-exchange resins, rhenium anions are exchanged with other

positively charged ions, enhancing the process efficiency [6].

Van der Waals Forces

: These forces, arising from molecular interactions, support the

adsorption of rhenium onto the sorbent surface [7].

Recent Research and Innovations

Recent years have witnessed significant research aimed at improving rhenium sorption methods.

Notable innovations include:

Nanomaterials

: New types of nanomaterials developed through nanotechnology offer

high surface areas and unique structures for effective rhenium adsorption [8].

Modified Polymers

: Sorption processes using polymer resins and nanomaterials are

being optimized to enhance efficiency [9].


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Biomass-Based Sorbents

: Newly developed sorbents based on natural biomass are both

eco-friendly and low-cost, representing a growing research area [10].

Conclusion

There are various materials and methods available for the effective sorption of rhenium.

Activated carbon, zeolites, ion-exchange resins, and modified biomass materials are widely used

in this field. In recent years, the development of more efficient sorption technologies using

nanomaterials and polymers has gained momentum. To reduce the environmental risks of

rhenium and ensure its effective removal from ecosystems, further development of these

methods is essential.

References

1.

Raha, S., & Ghosh, A. (2017).

Removal of perrhenate from aqueous solutions by

adsorption on activated carbon.

Journal of Environmental Chemical Engineering, 5(1), 1040–

1047.

2.

Benoit, J., & Schubert, T. (2015).

Perrhenate removal from aqueous solutions using

zeolites: An effective sorption approach.

Environmental Science & Technology, 49(22), 13556–

13564.

3.

Kim, H., & Lee, S. (2019).

Perrhenate adsorption on ion-exchange resins: A

comparative study of selectivity and efficiency.

Journal of Hazardous Materials, 380, 120848.

4.

Li, Z., & Liu, Q. (2020).

Adsorption of perrhenate from aqueous solutions using modified

carbon-based adsorbents.

Chemical Engineering Journal, 382, 122974.

5.

Patil, N., & Jadhav, S. (2021).

Effect of temperature and pH on perrhenate adsorption by

modified biosorbents.

Journal of Environmental Sciences, 95, 15–22.

6.

Sasaki, K., & Tanaka, N. (2018).

Sorption of rhenium and perrhenate onto ion-exchange

resins: A kinetic study.

Separation Science and Technology, 53(16), 2633–2643.

7.

Huang, S., & Xie, W. (2022).

Recent advances in the use of sorbents for rhenium and

perrhenate removal from aqueous solutions.

Environmental Pollution, 282, 117015.

8.

Chung, J., & Lee, M. (2016).

Removal of rhenium from aqueous solutions by adsorptive

materials: A review.

Journal of Environmental Management, 182, 340–350.

9.

N. Kattaev, B. Tuygun, D. Adinaeva, M. Jumaev, K. Azizova, A new granulated sorbent

based on acrylonitrile: Synthesis and physico-chemical properties, BIO Web Conferences, 95,

01043 (2024)

10.

Азизова Холида Мумин Кизи, Катаев Нуритдин Тураевич, Бабаев Туйгун

Мирзаахмедович ИССЛЕДОВАНИЕ ВЗАИМОДЕЙСТВИЯ ИОНОВ МЕДИ (II) С

НОВЫМ КОМПЛЕКСООБРАЗУЮЩИМ АНИОНИТОМ // Universum: химия и биология.

2021. №12-1 (90).

References

Raha, S., & Ghosh, A. (2017). Removal of perrhenate from aqueous solutions by adsorption on activated carbon. Journal of Environmental Chemical Engineering, 5(1), 1040–1047.

Benoit, J., & Schubert, T. (2015). Perrhenate removal from aqueous solutions using zeolites: An effective sorption approach. Environmental Science & Technology, 49(22), 13556–13564.

Kim, H., & Lee, S. (2019). Perrhenate adsorption on ion-exchange resins: A comparative study of selectivity and efficiency. Journal of Hazardous Materials, 380, 120848.

Li, Z., & Liu, Q. (2020). Adsorption of perrhenate from aqueous solutions using modified carbon-based adsorbents. Chemical Engineering Journal, 382, 122974.

Patil, N., & Jadhav, S. (2021). Effect of temperature and pH on perrhenate adsorption by modified biosorbents. Journal of Environmental Sciences, 95, 15–22.

Sasaki, K., & Tanaka, N. (2018). Sorption of rhenium and perrhenate onto ion-exchange resins: A kinetic study. Separation Science and Technology, 53(16), 2633–2643.

Huang, S., & Xie, W. (2022). Recent advances in the use of sorbents for rhenium and perrhenate removal from aqueous solutions. Environmental Pollution, 282, 117015.

Chung, J., & Lee, M. (2016). Removal of rhenium from aqueous solutions by adsorptive materials: A review. Journal of Environmental Management, 182, 340–350.

N. Kattaev, B. Tuygun, D. Adinaeva, M. Jumaev, K. Azizova, A new granulated sorbent based on acrylonitrile: Synthesis and physico-chemical properties, BIO Web Conferences, 95, 01043 (2024)

Азизова Холида Мумин Кизи, Катаев Нуритдин Тураевич, Бабаев Туйгун Мирзаахмедович ИССЛЕДОВАНИЕ ВЗАИМОДЕЙСТВИЯ ИОНОВ МЕДИ (II) С НОВЫМ КОМПЛЕКСООБРАЗУЮЩИМ АНИОНИТОМ // Universum: химия и биология. 2021. №12-1 (90).